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Au-198 shielding — lead half-value layer and dose rate

Gold-198

Au-198 · Gold, Z = 79, A = 198

At 9.06e+15 Bq/g — 2.45e+5 Ci/g — a gigabecquerel of Au-198 amounts to 110 ng, which is why activity rather than mass is how anyone states the quantity. Gold-198 decays by beta-minus decay with a half-life of 2.6941 days, falling to 16.51% of today's activity in a week and 6.8e-9% in three months.

1 GBq at 1 m reads 0.0546 mGy/h, and 1 Ci at the same distance 2.02 mGy/h, from an air kerma rate constant of 0.0546 mGy·m²/(GBq·h) — 1.4× less than Cs-137 and 5.6× less than Co-60, and 39 of 96 among the photon emitters carried here.

8 lines clear the 20 keV cutoff, but one of them carries 90% of the dose rate. The leading one is 411.8 keV at 97.7% of the total — its emission probability is 95.62%, which is also the highest.

Halving the air kerma rate calls for 2.77 mm of lead, or 9.47 mm of steel where lead is unwelcome, and a factor of ten calls for 9.32 mm of lead — sheet thicknesses that a glovebox or a transport container can carry. Reaching 20 µSv/h from 1 GBq at a metre takes 4.02 mm of lead.

Half-life, specific activity and dose rate

Half-life2.6941 days (2.328e+5 s)
Decay modebeta-minus decay
Specific activity9.06e+15 Bq/g (2.45e+5 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.0546 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.0546 mGy/h
Dose rate, 1 Ci at 1 m2.02 mGy/h
Kerma-weighted mean photon energy416.2 keV

412 keV carries 98% of the dose rate

1 further line below the 20 keV cutoff, the highest at 11.78 keV and 1.19% emission probability in all, is excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
411.8095.6297.72
675.880.805121.34
1087.680.158920.40
70.821.368830.22
68.890.807470.13
81.280.600660.10
80.320.464550.08
82.480.136110.02

2.77 mm of lead halves this spectrum

Solved numerically across all 8 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead2.779.323.37
tungsten1.956.583.36
iron9.4731.73.34
copper8.3227.83.34
concrete31.21043.33
water66.22203.33
aluminum28.093.43.33

A single energy would give 3.32. What a spread of energies does instead.

Activity over days and weeks

Ten half-lives is 26.9 days — a storage problem rather than a disposal one, with 1.5e-39% of today's activity still there after a year. The mean life 1/λ is 3.89 days.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity8.95 days
Time to fall to 1 %17.9 days
Time to fall to 0.1 %26.8 days

Limits of these dose rates

Gamma and decay calculators for Au-198

Other Gold nuclides: Au-198m

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.