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Ba-133 shielding — lead half-value layer and dose rate

Barium-133

Ba-133 · Barium, Z = 56, A = 133

Barium-133 decays by electron capture, half-life 10.551 years. Specific activity is 9.43e+12 Bq/g (255 Ci/g), so a gigabecquerel comes to 106 µg — weighable, but on an analytical balance. Over a year the activity falls to 93.64%, and over forty years to 7.22%.

1 GBq at 1 m reads 0.0733 mGy/h, and 1 Ci at the same distance 2.71 mGy/h, from an air kerma rate constant of 0.0733 mGy·m²/(GBq·h) — 1.1× less than Cs-137 and 4.2× less than Co-60, and 29 of 96 among the photon emitters carried here.

14 lines clear the 20 keV cutoff, but 7 of them carry 90% of the dose rate. The leading one is 356.0 keV at 40.4% of the total — its emission probability is 62.05%, which is also the highest.

A half-value layer of 0.582 mm in lead puts this in foil and thin sheet, with 2.69 mm needed if the material is steel; ten-fold attenuation comes at 5.16 mm of lead. Reaching 20 µSv/h from 1 GBq at a metre takes 2.25 mm of lead. The tenth-value layer runs 8.9 times the half-value layer, not the 3.32 a single energy would give.

Half-life, specific activity and dose rate

Half-life10.551 years (3.330e+8 s)
Decay modeelectron capture
Specific activity9.43e+12 Bq/g (255 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.0733 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.0733 mGy/h
Dose rate, 1 Ci at 1 m2.71 mGy/h
Kerma-weighted mean photon energy223.4 keV

14 lines above the cutoff, and what each contributes

1 further line below the 20 keV cutoff, the highest at 4.75 keV and 15.3% emission probability in all, is excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
356.0162.0540.37
30.9760.216.41
302.8518.3357810.00
30.6332.69.07
383.858.94146.32
35.4121.94.68
81.0032.948554.02
35.0917.63.82
276.407.160573.51
35.824.290.90
79.612.649540.32
53.162.140730.26
223.240.452970.17
160.610.637870.16

0.582 mm of lead halves this spectrum

Solved numerically across all 14 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead0.5825.168.88
tungsten0.3843.729.70
iron2.6922.48.33
copper2.2719.58.59
concrete12.975.95.88
water39.31634.16
aluminum10.868.16.27

A single energy would give 3.32. What a spread of energies does instead.

Activity over decades and centuries

Ten half-lives is 106 years, which puts decay storage out of reach: 7.22% survives forty years. The mean life 1/λ, the quantity that enters an integrated dose, is 15.2 years.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity35.0 years
Time to fall to 1 %70.1 years
Time to fall to 0.1 %105 years

Limits of these dose rates

Gamma and decay calculators for Ba-133

Other Barium nuclides: Ba-133m, Ba-137m

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.