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Eu-152 shielding — lead half-value layer and dose rate

Europium-152

Eu-152 · Europium, Z = 63, A = 152

Europium-152 decays by electron capture with beta-plus, half-life 13.517 years. Specific activity is 6.44e+12 Bq/g (174 Ci/g), so a gigabecquerel comes to 155 µg — weighable, but on an analytical balance. Over a year the activity falls to 95.00%, and over forty years to 12.86%.

1 GBq at 1 m reads 0.152 mGy/h, and 1 Ci at the same distance 5.63 mGy/h, from an air kerma rate constant of 0.152 mGy·m²/(GBq·h) — 2.0× Cs-137 and 2.0× less than Co-60, and 12 of 96 among the photon emitters carried here.

58 lines clear the 20 keV cutoff, but 15 of them carry 90% of the dose rate. The leading one is 1408.0 keV at 22.9% of the total — its emission probability is 20.87%, which is also the highest.

This is a shield that has to be designed: 6.24 mm of lead for a factor of two and 27.7 mm for a factor of ten, or 12.1 mm of steel to halve it, at which point the mass of the shield is part of the problem. Reaching 20 µSv/h from 1 GBq at a metre takes 23.9 mm of lead. The tenth-value layer runs 4.4 times the half-value layer, not the 3.32 a single energy would give.

Half-life, specific activity and dose rate

Half-life13.517 years (4.266e+8 s)
Decay modeelectron capture with beta-plus
Specific activity6.44e+12 Bq/g (174 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.152 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.152 mGy/h
Dose rate, 1 Ci at 1 m5.63 mGy/h
Kerma-weighted mean photon energy924.9 keV

58 lines above the cutoff, and what each contributes

2 further lines below the 20 keV cutoff, the highest at 6.86 keV and 14.2% emission probability in all, are excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
1408.0120.8722.92
1112.0813.6712.51
964.0614.5111.82
1085.8410.119.08
778.9012.938.77
344.2826.598.03
867.384.233.15
40.1237.83.10
121.7828.532.52
39.5220.871.76
1299.141.6331.69
1089.741.7341.56
244.707.551.54
1212.951.4151.39

Showing the 14 largest contributors of 58 lines above the cutoff; the remainder together carry 10.17% of the dose rate.

6.24 mm of lead halves this spectrum

Solved numerically across all 58 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead6.2427.74.43
tungsten3.9917.34.34
iron12.146.63.84
copper10.841.63.86
concrete39.51483.75
water85.53133.66
aluminum35.41333.76

A single energy would give 3.32. What a spread of energies does instead.

Activity over decades and centuries

Ten half-lives is 135 years, which puts decay storage out of reach: 12.86% survives forty years. The mean life 1/λ, the quantity that enters an integrated dose, is 19.5 years.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity44.9 years
Time to fall to 1 %89.8 years
Time to fall to 0.1 %135 years

Limits of these dose rates

Gamma and decay calculators for Eu-152

Other Europium nuclides: Eu-152m1, Eu-152m2, Eu-154, Eu-154m

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.