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Fe-59 shielding — lead half-value layer and dose rate

Iron-59

Fe-59 · Iron, Z = 26, A = 59

At 1.84e+15 Bq/g — 4.98e+4 Ci/g — a gigabecquerel of Fe-59 amounts to 543 ng, which is why activity rather than mass is how anyone states the quantity. Iron-59 decays by beta-minus decay with a half-life of 44.490 days, falling to 62.66% of today's activity in a month and 0.34% in a year.

1 GBq at 1 m reads 0.147 mGy/h, and 1 Ci at the same distance 5.43 mGy/h, from an air kerma rate constant of 0.147 mGy·m²/(GBq·h) — 1.9× Cs-137 and 2.1× less than Co-60, and 13 of 96 among the photon emitters carried here.

8 lines clear the 20 keV cutoff, but 2 of them carry 90% of the dose rate. The leading one is 1099.2 keV at 53.1% of the total — its emission probability is 56.5%, which is also the highest.

This is a shield that has to be designed: 9.80 mm of lead for a factor of two and 32.9 mm for a factor of ten, or 15.9 mm of steel to halve it, at which point the mass of the shield is part of the problem. Reaching 20 µSv/h from 1 GBq at a metre takes 28.4 mm of lead.

Half-life, specific activity and dose rate

Half-life44.490 days (3.844e+6 s)
Decay modebeta-minus decay
Specific activity1.84e+15 Bq/g (4.98e+4 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.147 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.147 mGy/h
Dose rate, 1 Ci at 1 m5.43 mGy/h
Kerma-weighted mean photon energy1182 keV

1099 keV leads, and 2 lines make 90%

3 further lines below the 20 keV cutoff, the highest at 7.68 keV and 0.0212% emission probability in all, are excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
1099.2456.553.12
1291.5943.246.12
192.343.080.49
142.651.020.11
334.800.270.08
1481.700.0590.07
382.000.0180.01
189.000.00110.00

9.80 mm of lead halves this spectrum

Solved numerically across all 8 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead9.8032.93.36
tungsten6.1020.53.35
iron15.953.13.34
copper14.247.43.34
concrete50.21683.34
water1063543.33
aluminum45.21513.34

A single energy would give 3.32. What a spread of energies does instead.

Activity over months and years

Ten half-lives is 1.22 years — a storage problem rather than a disposal one, with 0.34% of today's activity still there after a year. The mean life 1/λ is 64.2 days.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity148 days
Time to fall to 1 %296 days
Time to fall to 0.1 %1.21 years

Limits of these dose rates

Gamma and decay calculators for Fe-59

Other Iron nuclides: Fe-55

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.