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Pr-144 beta shielding — range and bremsstrahlung

Praseodymium-144

Pr-144 · Praseodymium, Z = 59, A = 144

Praseodymium-144 (Pr-144) carries 2.80e+18 Bq/g, or 7.56e+7 Ci/g: a gigabecquerel is 357 pg, no weighable quantity at all. It decays by beta-minus decay with a half-life of 17.28 minutes, which leaves 8.2e-24% of today's activity after a day and 2.5e-174% after a week.

The beta endpoint is 3.00 MeV, mean 1.21 MeV over 5 branches. That endpoint stops in 12.6 mm of acrylic or 5.93 mm of glass. Of the beta energy, 0.63% turns into X-rays in acrylic and 8.60% in lead.

Decay is the only handle: a day leaves 8.2e-24% of today's activity and a week leaves 2.5e-174%, with ten half-lives at 2.88 hours and a mean life of 24.9 minutes per atom.

Half-life, specific activity and beta endpoint

Half-life17.28 minutes (1037 s)
Decay modebeta-minus decay
Specific activity2.80e+18 Bq/g (7.56e+7 Ci/g)
Beta endpoint / mean3.00 MeV / 1.21 MeV

12.6 mm of acrylic stops the 3.00 MeV endpoint

Katz–Penfold fit to the 3.00 MeV endpoint — ±10%, and a stopping thickness rather than an attenuation length. Why the material matters more than the thickness.

AbsorberRange for the endpoint (mm)
acrylic12.6
aluminum5.49
water14.8
glass5.93
Shield materialFraction of beta energy converted to X-rays
acrylic (Z ≈ 6)0.63%
lead (Z = 82)8.60%

Activity over the first hours

Ten half-lives is 2.88 hours, so the activity moves measurably while a count is running: every figure has to carry the time it was referred to. The mean life 1/λ is 24.9 minutes.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity57.4 minutes
Time to fall to 1 %1.91 hours
Time to fall to 0.1 %2.87 hours

Limits of these range figures

Beta and decay calculators for Pr-144

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.