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Pu-241 beta shielding — range and bremsstrahlung

Plutonium-241

Pu-241 · Plutonium, Z = 94, A = 241

Plutonium-241 decays by alpha decay, half-life 14.329 years. Specific activity is 3.83e+12 Bq/g (104 Ci/g), so a gigabecquerel comes to 261 µg — weighable, but on an analytical balance. Over a year the activity falls to 95.28%, and over forty years to 14.44%.

All 1 recorded photon lines sit below the 20 keV cutoff, so Γ is zero by convention and no external dose rate is quoted. The strongest line is 16.68 keV. A monitor calibrated on Cs-137 under-responds at these energies, so a reading taken without an energy correction understates Pu-241 rather than missing it outright. The recorded spectrum runs 16.7 to 16.7 keV and carries 0.00125% emission probability in all, which sets what a thin-window or proportional detector has to see.

The beta endpoint is 0.0208 MeV, mean 0.00523 MeV over 1 branch. That endpoint stops in 0.00621 mm of acrylic or 0.00293 mm of glass. Of the beta energy, 4.4e-3% turns into X-rays in acrylic and 0.06% in lead.

Decay is the only handle: a year leaves 95.28% of today's activity and forty years leaves 14.44%, with ten half-lives at 143 years and a mean life of 20.7 years per atom.

Half-life, specific activity and beta endpoint

Half-life14.329 years (4.522e+8 s)
Decay modealpha decay
Specific activity3.83e+12 Bq/g (104 Ci/g)
Beta endpoint / mean0.0208 MeV / 0.00523 MeV

0.00621 mm of acrylic stops the 0.0208 MeV endpoint

Katz–Penfold fit to the 0.0208 MeV endpoint — ±10%, and a stopping thickness rather than an attenuation length. Why the material matters more than the thickness.

AbsorberRange for the endpoint (mm)
acrylic0.00621
aluminum0.00272
water0.00733
glass0.00293
Shield materialFraction of beta energy converted to X-rays
acrylic (Z ≈ 6)0.00%
lead (Z = 82)0.06%

Activity over decades and centuries

Ten half-lives is 143 years, which puts decay storage out of reach: 14.44% survives forty years. The mean life 1/λ, the quantity that enters an integrated dose, is 20.7 years.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity47.6 years
Time to fall to 1 %95.2 years
Time to fall to 0.1 %143 years

Limits of these range figures

Beta and decay calculators for Pu-241

Other Plutonium nuclides: Pu-238, Pu-239, Pu-240, Pu-242, Pu-244

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.