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Rh-106 shielding — lead half-value layer and dose rate

Rhodium-106

Rh-106 · Rhodium, Z = 45, A = 106

Rhodium-106 (Rh-106) carries 1.31e+20 Bq/g, or 3.54e+9 Ci/g: a gigabecquerel is 7.63 pg, no weighable quantity at all. It decays by beta-minus decay with a half-life of 30.07 seconds, which leaves 0% of today's activity after a day and 0% after a week.

At 0.0275 mGy·m²/(GBq·h) the air kerma rate constant is 2.8× less than Cs-137 and 11× less than Co-60, placing it 50 of 96 photon emitters in this dataset. 1 GBq at 1 m reads 0.0275 mGy/h, and 1 Ci at the same distance 1.02 mGy/h.

59 lines clear the 20 keV cutoff, but 4 of them carry 90% of the dose rate. The leading one is 511.9 keV at 51.6% of the total — its emission probability is 20.4%, which is also the highest.

Halving the air kerma rate calls for 4.79 mm of lead, or 11.5 mm of steel where lead is unwelcome, and a factor of ten calls for 17.2 mm of lead — sheet thicknesses that a glovebox or a transport container can carry. Reaching 20 µSv/h from 1 GBq at a metre takes 2.17 mm of lead.

The beta endpoint is 3.54 MeV, mean 1.41 MeV over 12 branches. That endpoint stops in 15.0 mm of acrylic or 7.08 mm of glass. Of the beta energy, 0.74% turns into X-rays in acrylic and 10.16% in lead.

Half-life, specific activity, dose rate and beta energies

Half-life30.07 seconds (30.07 s)
Decay modebeta-minus decay
Specific activity1.31e+20 Bq/g (3.54e+9 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.0275 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.0275 mGy/h
Dose rate, 1 Ci at 1 m1.02 mGy/h
Kerma-weighted mean photon energy653.7 keV
Beta endpoint / mean3.54 MeV / 1.41 MeV

59 lines above the cutoff, and what each contributes

1 further line below the 20 keV cutoff, the highest at 3.05 keV and 0.00711% emission probability in all, is excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
511.8620.451.59
621.939.934830.32
1050.411.558567.53
616.220.75482.28
1128.070.403922.07
873.490.43861.82
1562.250.16321.07
1194.540.057320.31
2112.540.034480.28
1766.250.034270.25
2366.040.023260.20
1988.440.026110.20
1796.940.027740.20
1062.140.032030.16

Showing the 14 largest contributors of 59 lines above the cutoff; the remainder together carry 1.73% of the dose rate.

4.79 mm of lead halves this spectrum

Solved numerically across all 59 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead4.7917.23.59
tungsten3.2211.43.54
iron11.539.03.39
copper10.234.63.39
concrete37.01253.38
water78.32653.38
aluminum33.31133.38

A single energy would give 3.32. What a spread of energies does instead.

15.0 mm of acrylic stops the 3.54 MeV endpoint

Katz–Penfold fit to the 3.54 MeV endpoint — ±10%, and a stopping thickness rather than an attenuation length. Why the material matters more than the thickness.

AbsorberRange for the endpoint (mm)
acrylic15.0
aluminum6.56
water17.7
glass7.08
Shield materialFraction of beta energy converted to X-rays
acrylic (Z ≈ 6)0.74%
lead (Z = 82)10.16%

Activity over the first hours

Ten half-lives is 5.01 minutes, so the activity moves measurably while a count is running: every figure has to carry the time it was referred to. The mean life 1/λ is 43.4 seconds.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity1.66 minutes
Time to fall to 1 %3.33 minutes
Time to fall to 0.1 %4.99 minutes

Limits of these dose rates

Gamma, beta and decay calculators for Rh-106

Other Rhodium nuclides: Rh-106m

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.