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Sm-153 shielding — lead half-value layer and dose rate

Samarium-153

Sm-153 · Samarium, Z = 62, A = 153

Samarium-153 (Sm-153) carries 1.64e+16 Bq/g, or 4.43e+5 Ci/g: a gigabecquerel is 61.0 ng, no weighable quantity at all. It decays by beta-minus decay with a half-life of 46.284 hours, which leaves 8.08% of today's activity after a week and 6.2e-13% after three months.

At 0.0119 mGy·m²/(GBq·h) the air kerma rate constant is 6.5× less than Cs-137 and 26× less than Co-60, placing it 67 of 96 photon emitters in this dataset. 1 GBq at 1 m reads 0.0119 mGy/h, and 1 Ci at the same distance 0.441 mGy/h.

38 lines clear the 20 keV cutoff, but 5 of them carry 90% of the dose rate. The leading one is 41.5 keV at 30.1% of the total — its emission probability is 30.03632%, which is also the highest.

Shielding barely arises: 0.0673 mm of lead halves the air kerma rate and 0.274 mm takes it to a tenth, thicknesses a source capsule is likely to exceed on its own. Steel does the halving in 0.485 mm. At 1 GBq and a metre it is already under 20 µSv/h with nothing in the way. The tenth-value layer runs 4.1 times the half-value layer, not the 3.32 a single energy would give.

Half-life, specific activity and dose rate

Half-life46.284 hours (1.666e+5 s)
Decay modebeta-minus decay
Specific activity1.64e+16 Bq/g (4.43e+5 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.0119 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.0119 mGy/h
Dose rate, 1 Ci at 1 m0.441 mGy/h
Kerma-weighted mean photon energy66.54 keV

38 lines above the cutoff, and what each contributes

1 further line below the 20 keV cutoff, the highest at 6.60 keV and 10.7% emission probability in all, is excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
41.5430.0363230.11
103.1829.1427.07
40.9016.6461317.03
47.6511.9040210.00
47.159.462668.06
69.674.668233.37
48.252.441372.02
97.430.763470.67
531.400.054670.33
533.200.029550.18
83.370.190870.15
75.420.192320.14
89.490.157360.13
539.100.020660.13

Showing the 14 largest contributors of 38 lines above the cutoff; the remainder together carry 0.62% of the dose rate.

0.0673 mm of lead halves this spectrum

Solved numerically across all 38 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead0.06730.2744.07
tungsten0.04990.1933.88
iron0.4854.138.52
copper0.3222.969.20
concrete8.9135.43.97
water31.01073.44
aluminum7.0529.54.18

A single energy would give 3.32. What a spread of energies does instead.

Activity over days and weeks

Ten half-lives is 19.3 days — a storage problem rather than a disposal one, with 9.7e-56% of today's activity still there after a year. The mean life 1/λ is 2.78 days.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity6.41 days
Time to fall to 1 %12.8 days
Time to fall to 0.1 %19.2 days

Limits of these dose rates

Gamma and decay calculators for Sm-153

Other Samarium nuclides: Sm-147, Sm-151, Sm-153m

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.