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Tl-204 beta shielding — range and bremsstrahlung

Thallium-204

Tl-204 · Thallium, Z = 81, A = 204

Thallium-204 decays by beta-minus decay, half-life 3.783 years. Specific activity is 1.71e+13 Bq/g (463 Ci/g), so a gigabecquerel comes to 58.3 µg — weighable, but on an analytical balance. Over a year the activity falls to 83.26%, and over forty years to 0.07%.

The beta endpoint is 0.763 MeV, mean 0.244 MeV over 1 branch. That endpoint stops in 2.46 mm of acrylic or 1.16 mm of glass. Of the beta energy, 0.16% turns into X-rays in acrylic and 2.19% in lead.

Decay is the only handle: a year leaves 83.26% of today's activity and forty years leaves 0.07%, with ten half-lives at 37.8 years and a mean life of 5.46 years per atom.

Half-life, specific activity and beta endpoint

Half-life3.783 years (1.194e+8 s)
Decay modebeta-minus decay
Specific activity1.71e+13 Bq/g (463 Ci/g)
Beta endpoint / mean0.763 MeV / 0.244 MeV

2.46 mm of acrylic stops the 0.763 MeV endpoint

Katz–Penfold fit to the 0.763 MeV endpoint — ±10%, and a stopping thickness rather than an attenuation length. Why the material matters more than the thickness.

AbsorberRange for the endpoint (mm)
acrylic2.46
aluminum1.08
water2.91
glass1.16
Shield materialFraction of beta energy converted to X-rays
acrylic (Z ≈ 6)0.16%
lead (Z = 82)2.19%

Activity over decades and centuries

Ten half-lives is 37.8 years, which puts decay storage out of reach: 0.07% survives forty years. The mean life 1/λ, the quantity that enters an integrated dose, is 5.46 years.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.12 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity12.6 years
Time to fall to 1 %25.1 years
Time to fall to 0.1 %37.7 years

Limits of these range figures

Beta and decay calculators for Tl-204

Other Thallium nuclides: Tl-201, Tl-201m

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.