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Y-90m shielding — lead half-value layer and dose rate

Yttrium-90m

Y-90m · Yttrium, Z = 39, A = 90 · isomeric state m

Yttrium-90m (Y-90m) carries 4.04e+17 Bq/g, or 1.09e+7 Ci/g: a gigabecquerel is 2.47 ng, no weighable quantity at all. It decays by isomeric transition with a half-life of 3.19 hours, which leaves 0.54% of today's activity after a day and 1.4e-14% after a week.

1 GBq at 1 m reads 0.0835 mGy/h, and 1 Ci at the same distance 3.09 mGy/h, from an air kerma rate constant of 0.0835 mGy·m²/(GBq·h) — 1.1× Cs-137 and 3.7× less than Co-60, and 25 of 96 among the photon emitters carried here.

4 lines clear the 20 keV cutoff, but 2 of them carry 90% of the dose rate. The leading one is 479.5 keV at 70.7% of the total — its emission probability is 90.5%, which is lower than the 97% of the 202.5 keV line it outranks.

Halving the air kerma rate calls for 2.10 mm of lead, or 8.75 mm of steel where lead is unwelcome, and a factor of ten calls for 10.0 mm of lead — sheet thicknesses that a glovebox or a transport container can carry. Reaching 20 µSv/h from 1 GBq at a metre takes 5.57 mm of lead. The tenth-value layer runs 4.8 times the half-value layer, not the 3.32 a single energy would give.

Half-life, specific activity and dose rate

Half-life3.19 hours (1.148e+4 s)
Decay modeisomeric transition
Specific activity4.04e+17 Bq/g (1.09e+7 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.0835 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.0835 mGy/h
Dose rate, 1 Ci at 1 m3.09 mGy/h
Kerma-weighted mean photon energy400.2 keV

480 keV leads, and 2 lines make 90%

6 further lines below the 20 keV cutoff, the highest at 17.01 keV and 8.47% emission probability in all, are excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
479.5190.570.71
202.539728.93
681.800.320.35
2318.970.00180.01

2.10 mm of lead halves this spectrum

Solved numerically across all 4 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead2.1010.04.78
tungsten1.486.944.68
iron8.7530.43.48
copper7.5626.63.52
concrete30.01023.39
water63.92163.38
aluminum26.991.33.39

A single energy would give 3.32. What a spread of energies does instead.

Activity over days and weeks

Ten half-lives is 1.33 days, so the activity moves measurably while a count is running: every figure has to carry the time it was referred to. The mean life 1/λ is 4.60 hours.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity10.6 hours
Time to fall to 1 %21.2 hours
Time to fall to 0.1 %1.32 days

Limits of these dose rates

Gamma and decay calculators for Y-90m

Other Yttrium nuclides: Y-88, Y-88m1, Y-88m2, Y-90, Y-91

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.