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Au-198m shielding — lead half-value layer and dose rate

Gold-198m

Au-198m · Gold, Z = 79, A = 198 · isomeric state m

Gold-198m (Au-198m) carries 1.07e+16 Bq/g, or 2.90e+5 Ci/g: a gigabecquerel is 93.1 ng, no weighable quantity at all. It decays by isomeric transition with a half-life of 2.272 days, which leaves 11.82% of today's activity after a week and 8.8e-11% after three months.

1 GBq at 1 m reads 0.0647 mGy/h, and 1 Ci at the same distance 2.39 mGy/h, from an air kerma rate constant of 0.0647 mGy·m²/(GBq·h) — 1.2× less than Cs-137 and 4.7× less than Co-60, and 35 of 96 among the photon emitters carried here.

11 lines clear the 20 keV cutoff, but 6 of them carry 90% of the dose rate. The leading one is 214.9 keV at 31.8% of the total — its emission probability is 77%, which is also the highest.

A half-value layer of 0.481 mm in lead puts this in foil and thin sheet, with 4.46 mm needed if the material is steel; ten-fold attenuation comes at 2.36 mm of lead. Reaching 20 µSv/h from 1 GBq at a metre takes 0.960 mm of lead. The tenth-value layer runs 4.9 times the half-value layer, not the 3.32 a single energy would give.

Half-life, specific activity and dose rate

Half-life2.272 days (1.963e+5 s)
Decay modeisomeric transition
Specific activity1.07e+16 Bq/g (2.90e+5 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.0647 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.0647 mGy/h
Dose rate, 1 Ci at 1 m2.39 mGy/h
Kerma-weighted mean photon energy189.5 keV

11 lines above the cutoff, and what each contributes

1 further line below the 20 keV cutoff, the highest at 11.42 keV and 57.3% emission probability in all, is excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
214.897731.76
180.3149.2816.43
204.1038.514.94
333.8217.7112.16
97.2168.5311.03
68.8141.557325.52
66.9924.410773.22
78.9818.075262.46
78.0514.02271.91
80.134.052560.55
115.200.040040.01

0.481 mm of lead halves this spectrum

Solved numerically across all 11 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead0.4812.364.90
tungsten0.3441.755.08
iron4.4618.84.21
copper3.5615.64.38
concrete21.574.33.46
water48.21633.39
aluminum18.966.13.49

A single energy would give 3.32. What a spread of energies does instead.

Activity over days and weeks

Ten half-lives is 22.7 days — a storage problem rather than a disposal one, with 4.0e-47% of today's activity still there after a year. The mean life 1/λ is 3.28 days.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity7.55 days
Time to fall to 1 %15.1 days
Time to fall to 0.1 %22.6 days

Limits of these dose rates

Gamma and decay calculators for Au-198m

Other Gold nuclides: Au-198

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.