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Ga-67 shielding — lead half-value layer and dose rate

Gallium-67

Ga-67 · Gallium, Z = 31, A = 67

Gallium-67 (Ga-67) carries 2.21e+16 Bq/g, or 5.98e+5 Ci/g: a gigabecquerel is 45.2 ng, no weighable quantity at all. It decays by electron capture with a half-life of 3.2617 days, which leaves 22.59% of today's activity after a week and 4.0e-7% after three months.

At 0.0189 mGy·m²/(GBq·h) the air kerma rate constant is 4.1× less than Cs-137 and 16× less than Co-60, placing it 55 of 96 photon emitters in this dataset. 1 GBq at 1 m reads 0.0189 mGy/h, and 1 Ci at the same distance 0.699 mGy/h.

10 lines clear the 20 keV cutoff, but 4 of them carry 90% of the dose rate. The leading one is 300.2 keV at 34.8% of the total — its emission probability is 16.64%, which is lower than the 21.41% of the 184.6 keV line it outranks.

A half-value layer of 0.656 mm in lead puts this in foil and thin sheet, with 5.36 mm needed if the material is steel; ten-fold attenuation comes at 4.28 mm of lead. At 1 GBq and a metre it is already under 20 µSv/h with nothing in the way. The tenth-value layer runs 6.5 times the half-value layer, not the 3.32 a single energy would give.

Half-life, specific activity and dose rate

Half-life3.2617 days (2.818e+5 s)
Decay modeelectron capture
Specific activity2.21e+16 Bq/g (5.98e+5 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.0189 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.0189 mGy/h
Dose rate, 1 Ci at 1 m0.699 mGy/h
Kerma-weighted mean photon energy241.4 keV

10 lines above the cutoff, and what each contributes

4 further lines below the 20 keV cutoff, the highest at 9.61 keV and 59.6% emission probability in all, are excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
300.2216.6434.85
184.5821.4125.16
93.3138.8120.67
393.534.5612.83
208.952.463.36
91.273.111.63
887.690.1480.91
794.380.0540.30
494.170.06840.24
703.110.01050.05

0.656 mm of lead halves this spectrum

Solved numerically across all 10 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead0.6564.286.52
tungsten0.4843.106.39
iron5.3622.14.12
copper4.3518.84.33
concrete23.681.63.46
water51.91773.41
aluminum20.972.83.48

A single energy would give 3.32. What a spread of energies does instead.

Activity over months and years

Ten half-lives is 32.6 days — a storage problem rather than a disposal one, with 2.0e-32% of today's activity still there after a year. The mean life 1/λ is 4.71 days.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity10.8 days
Time to fall to 1 %21.7 days
Time to fall to 0.1 %32.5 days

Limits of these dose rates

Gamma and decay calculators for Ga-67

Other Gallium nuclides: Ga-68

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.