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Ga-68 shielding — lead half-value layer and dose rate

Gallium-68

Ga-68 · Gallium, Z = 31, A = 68

Gallium-68 (Ga-68) carries 1.51e+18 Bq/g, or 4.09e+7 Ci/g: a gigabecquerel is 661 pg, no weighable quantity at all. It decays by electron capture with beta-plus with a half-life of 67.71 minutes, which leaves 4.0e-5% of today's activity after a day and 1.5e-43% after a week.

1 GBq at 1 m reads 0.129 mGy/h, and 1 Ci at the same distance 4.76 mGy/h, from an air kerma rate constant of 0.129 mGy·m²/(GBq·h) — 1.7× Cs-137 and 2.4× less than Co-60, and 16 of 96 among the photon emitters carried here.

8 lines clear the 20 keV cutoff, but one of them carries 90% of the dose rate. The leading one is 511.0 keV at 96.2% of the total — its emission probability is 177.82052%, which is also the highest.

Halving the air kerma rate calls for 4.01 mm of lead, or 10.7 mm of steel where lead is unwelcome, and a factor of ten calls for 13.6 mm of lead — sheet thicknesses that a glovebox or a transport container can carry. Reaching 20 µSv/h from 1 GBq at a metre takes 10.9 mm of lead.

Half-life, specific activity and dose rate

Half-life67.71 minutes (4063 s)
Decay modeelectron capture with beta-plus
Specific activity1.51e+18 Bq/g (4.09e+7 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.129 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.129 mGy/h
Dose rate, 1 Ci at 1 m4.76 mGy/h
Kerma-weighted mean photon energy534.6 keV

511 keV carries 96% of the dose rate

4 further lines below the 20 keV cutoff, the highest at 9.61 keV and 4.92% emission probability in all, are excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
511.00177.8205296.15
1077.343.223.40
1883.160.136530.22
1261.080.094350.11
805.830.094020.08
578.520.033490.02
1744.420.00950.01
2338.440.001130.00

4.01 mm of lead halves this spectrum

Solved numerically across all 8 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead4.0113.63.39
tungsten2.759.283.38
iron10.735.83.34
copper9.4931.73.34
concrete34.61153.33
water73.22443.33
aluminum31.11043.33

A single energy would give 3.32. What a spread of energies does instead.

Activity over the first hours

Ten half-lives is 11.3 hours, so the activity moves measurably while a count is running: every figure has to carry the time it was referred to. The mean life 1/λ is 1.63 hours.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity3.75 hours
Time to fall to 1 %7.50 hours
Time to fall to 0.1 %11.2 hours

Limits of these dose rates

Gamma and decay calculators for Ga-68

Other Gallium nuclides: Ga-67

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.