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Lu-177 shielding — lead half-value layer and dose rate

Lutetium-177

Lu-177 · Lutetium, Z = 71, A = 177

At 4.11e+15 Bq/g — 1.11e+5 Ci/g — a gigabecquerel of Lu-177 amounts to 243 ng, which is why activity rather than mass is how anyone states the quantity. Lutetium-177 decays by beta-minus decay with a half-life of 6.6443 days, falling to 48.18% of today's activity in a week and 7.5e-3% in three months.

The air kerma rate constant is small — 0.00420 mGy·m²/(GBq·h), 18× less than Cs-137 and 73× less than Co-60, ranking 77 of 96 by Γ — near the bottom of the photon emitters, but above the cutoff, which 51 nuclides in this dataset are not. 1 GBq at 1 m reads 0.00420 mGy/h, and 1 Ci at the same distance 0.155 mGy/h. It takes 4.76 GBq at a metre to reach 20 µSv/h from the photons alone.

11 lines clear the 20 keV cutoff, but 4 of them carry 90% of the dose rate. The leading one is 208.4 keV at 63.8% of the total — its emission probability is 10.41%, which is also the highest.

A half-value layer of 0.391 mm in lead puts this in foil and thin sheet, with 4.11 mm needed if the material is steel; ten-fold attenuation comes at 1.94 mm of lead. At 1 GBq and a metre it is already under 20 µSv/h with nothing in the way. The tenth-value layer runs 5.0 times the half-value layer, not the 3.32 a single energy would give.

Half-life, specific activity and dose rate

Half-life6.6443 days (5.741e+5 s)
Decay modebeta-minus decay
Specific activity4.11e+15 Bq/g (1.11e+5 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.00420 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.00420 mGy/h
Dose rate, 1 Ci at 1 m0.155 mGy/h
Kerma-weighted mean photon energy172.9 keV

11 lines above the cutoff, and what each contributes

1 further line below the 20 keV cutoff, the highest at 9.11 keV and 3.04% emission probability in all, is excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
208.3710.4163.79
112.956.2318.26
55.792.750445.74
54.611.57163.33
64.061.149662.32
321.320.21862.22
63.330.907391.83
249.670.19971.51
64.940.242270.49
71.640.1640.34
136.720.04650.17

0.391 mm of lead halves this spectrum

Solved numerically across all 11 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead0.3911.944.96
tungsten0.2931.454.94
iron4.1117.64.28
copper3.2814.54.42
concrete20.371.53.52
water46.61583.39
aluminum17.863.63.57

A single energy would give 3.32. What a spread of energies does instead.

Activity over months and years

Ten half-lives is 66.4 days — a storage problem rather than a disposal one, with 2.8e-15% of today's activity still there after a year. The mean life 1/λ is 9.59 days.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity22.1 days
Time to fall to 1 %44.1 days
Time to fall to 0.1 %66.2 days

Limits of these dose rates

Gamma and decay calculators for Lu-177

Other Lutetium nuclides: Lu-177m

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.