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Lu-177m shielding — lead half-value layer and dose rate

Lutetium-177m

Lu-177m · Lutetium, Z = 71, A = 177 · isomeric state m

At 1.70e+14 Bq/g — 4.60e+3 Ci/g — a gigabecquerel of Lu-177m amounts to 5.87 µg, which is why activity rather than mass is how anyone states the quantity. Lutetium-177m decays by beta-minus decay with a half-life of 160.4 days, falling to 87.84% of today's activity in a month and 20.63% in a year.

1 GBq at 1 m reads 0.131 mGy/h, and 1 Ci at the same distance 4.86 mGy/h, from an air kerma rate constant of 0.131 mGy·m²/(GBq·h) — 1.7× Cs-137 and 2.3× less than Co-60, and 15 of 96 among the photon emitters carried here.

57 lines clear the 20 keV cutoff, but 26 of them carry 90% of the dose rate. The leading one is 378.5 keV at 11.4% of the total — its emission probability is 29.4%, which is lower than the 55.4% of the 208.4 keV line it outranks.

A half-value layer of 0.926 mm in lead puts this in foil and thin sheet, with 5.94 mm needed if the material is steel; ten-fold attenuation comes at 5.33 mm of lead. Reaching 20 µSv/h from 1 GBq at a metre takes 3.99 mm of lead. The tenth-value layer runs 5.8 times the half-value layer, not the 3.32 a single energy would give.

Half-life, specific activity and dose rate

Half-life160.4 days (1.386e+7 s)
Decay modebeta-minus decay
Specific activity1.70e+14 Bq/g (4.60e+3 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.131 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.131 mGy/h
Dose rate, 1 Ci at 1 m4.86 mGy/h
Kerma-weighted mean photon energy267.7 keV

57 lines above the cutoff, and what each contributes

3 further lines below the 20 keV cutoff, the highest at 14.05 keV and 53.2% emission probability in all, are excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
378.5029.411.42
208.3755.410.87
418.5421.729.39
228.4835.97.85
413.6617.627.52
327.6818.436.12
281.7913.973.91
55.7957.798573.86
319.0210.513.39
204.1013.512.59
54.6133.02612.24
153.2816.542.22
112.9521.42.01
174.4012.471.97

Showing the 14 largest contributors of 57 lines above the cutoff; the remainder together carry 24.65% of the dose rate.

0.926 mm of lead halves this spectrum

Solved numerically across all 57 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead0.9265.335.75
tungsten0.6783.815.62
iron5.9424.14.05
copper5.0020.74.14
concrete23.985.23.57
water53.41843.44
aluminum21.176.33.61

A single energy would give 3.32. What a spread of energies does instead.

Activity over months and years

Ten half-lives is 4.39 years — a storage problem rather than a disposal one, with 20.63% of today's activity still there after a year. The mean life 1/λ is 231 days.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity1.46 years
Time to fall to 1 %2.92 years
Time to fall to 0.1 %4.38 years

Limits of these dose rates

Gamma and decay calculators for Lu-177m

Other Lutetium nuclides: Lu-177

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.