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Sm-153m shielding — lead half-value layer and dose rate

Samarium-153m

Sm-153m · Samarium, Z = 62, A = 153 · isomeric state m

Samarium-153m (Sm-153m) carries 2.58e+23 Bq/g, or 6.96e+12 Ci/g: a gigabecquerel is 3.88 fg, no weighable quantity at all. It decays by isomeric transition with a half-life of 10.6 milliseconds, which leaves 0% of today's activity after a day and 0% after a week.

At 0.0104 mGy·m²/(GBq·h) the air kerma rate constant is 7.4× less than Cs-137 and 29× less than Co-60, placing it 69 of 96 photon emitters in this dataset. 1 GBq at 1 m reads 0.0104 mGy/h, and 1 Ci at the same distance 0.385 mGy/h.

9 lines clear the 20 keV cutoff, but 2 of them carry 90% of the dose rate. The leading one is 32.9 keV at 86.1% of the total — its emission probability is 50.1%, which is also the highest.

Shielding barely arises: 0.0280 mm of lead halves the air kerma rate and 0.0982 mm takes it to a tenth, thicknesses a source capsule is likely to exceed on its own. Steel does the halving in 0.153 mm. At 1 GBq and a metre it is already under 20 µSv/h with nothing in the way.

Half-life, specific activity and dose rate

Half-life10.6 milliseconds (0.01060 s)
Decay modeisomeric transition
Specific activity2.58e+23 Bq/g (6.96e+12 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.0104 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.0104 mGy/h
Dose rate, 1 Ci at 1 m0.385 mGy/h
Kerma-weighted mean photon energy34.46 keV

32.9 keV carries 86% of the dose rate

3 further lines below the 20 keV cutoff, the highest at 11.90 keV and 28.2% emission probability in all, are excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
32.9050.186.08
40.123.750994.50
39.522.072422.55
46.102.20442.21
46.001.475071.48
45.521.172551.20
58.001.15230.95
53.600.85170.74
46.580.302520.30

0.0280 mm of lead halves this spectrum

Solved numerically across all 9 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead0.02800.09823.51
tungsten0.02200.07743.52
iron0.1530.5433.54
copper0.1010.3573.54
concrete4.1514.33.44
water21.471.63.35
aluminum3.0710.63.46

A single energy would give 3.32. What a spread of energies does instead.

Activity over the first hours

Ten half-lives is 0.106 seconds, so the activity moves measurably while a count is running: every figure has to carry the time it was referred to. The mean life 1/λ is 0.0153 seconds.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity0.0352 seconds
Time to fall to 1 %0.0704 seconds
Time to fall to 0.1 %0.106 seconds

Limits of these dose rates

Gamma and decay calculators for Sm-153m

Other Samarium nuclides: Sm-147, Sm-151, Sm-153

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.