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Ta-182 shielding — lead half-value layer and dose rate

Tantalum-182

Ta-182 · Tantalum, Z = 73, A = 182

At 2.31e+14 Bq/g — 6.25e+3 Ci/g — a gigabecquerel of Ta-182 amounts to 4.32 µg, which is why activity rather than mass is how anyone states the quantity. Tantalum-182 decays by beta-minus decay with a half-life of 114.74 days, falling to 83.42% of today's activity in a month and 11.01% in a year.

1 GBq at 1 m reads 0.162 mGy/h, and 1 Ci at the same distance 6.01 mGy/h, from an air kerma rate constant of 0.162 mGy·m²/(GBq·h) — 2.1× Cs-137 and 1.9× less than Co-60, and 10 of 96 among the photon emitters carried here.

48 lines clear the 20 keV cutoff, but 10 of them carry 90% of the dose rate. The leading one is 1121.3 keV at 30.4% of the total — its emission probability is 35.24%, which is also the highest.

This is a shield that has to be designed: 8.30 mm of lead for a factor of two and 31.3 mm for a factor of ten, or 13.8 mm of steel to halve it, at which point the mass of the shield is part of the problem. Reaching 20 µSv/h from 1 GBq at a metre takes 28.3 mm of lead.

Half-life, specific activity and dose rate

Half-life114.74 days (9.914e+6 s)
Decay modebeta-minus decay
Specific activity2.31e+14 Bq/g (6.25e+3 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.162 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.162 mGy/h
Dose rate, 1 Ci at 1 m6.01 mGy/h
Kerma-weighted mean photon energy1069 keV

48 lines above the cutoff, and what each contributes

1 further line below the 20 keV cutoff, the highest at 9.74 keV and 23.6% emission probability in all, is excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
1121.2935.2430.44
1221.3927.2299525.19
1189.0416.4852714.92
1231.0011.615110.81
67.7542.922322.27
1001.702.086211.65
1257.411.509331.43
1289.141.371891.32
222.117.566031.29
100.1114.201720.93
59.3217.461470.91
152.437.016280.76
264.073.61210.76
1157.300.732990.65

Showing the 14 largest contributors of 48 lines above the cutoff; the remainder together carry 6.67% of the dose rate.

8.30 mm of lead halves this spectrum

Solved numerically across all 48 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead8.3031.33.77
tungsten5.1719.53.76
iron13.850.53.65
copper12.345.13.66
concrete44.91603.55
water96.13373.51
aluminum40.31443.56

A single energy would give 3.32. What a spread of energies does instead.

Activity over months and years

Ten half-lives is 3.14 years — a storage problem rather than a disposal one, with 11.01% of today's activity still there after a year. The mean life 1/λ is 166 days.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity1.04 years
Time to fall to 1 %2.09 years
Time to fall to 0.1 %3.13 years

Limits of these dose rates

Gamma and decay calculators for Ta-182

Other Tantalum nuclides: Ta-182m1, Ta-182m2

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.