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Ta-182m2 shielding — lead half-value layer and dose rate

Tantalum-182m2

Ta-182m2 · Tantalum, Z = 73, A = 182 · isomeric state m2

Tantalum-182m2 (Ta-182m2) carries 2.41e+18 Bq/g, or 6.52e+7 Ci/g: a gigabecquerel is 414 pg, no weighable quantity at all. It decays by isomeric transition with a half-life of 15.84 minutes, which leaves 4.3e-26% of today's activity after a day and 2.7e-190% after a week.

At 0.0339 mGy·m²/(GBq·h) the air kerma rate constant is 2.3× less than Cs-137 and 9.0× less than Co-60, placing it 47 of 96 photon emitters in this dataset. 1 GBq at 1 m reads 0.0339 mGy/h, and 1 Ci at the same distance 1.25 mGy/h.

10 lines clear the 20 keV cutoff, but 7 of them carry 90% of the dose rate. The leading one is 171.6 keV at 28.7% of the total — its emission probability is 48%, which is also the highest.

A half-value layer of 0.297 mm in lead puts this in foil and thin sheet, with 2.97 mm needed if the material is steel; ten-fold attenuation comes at 1.47 mm of lead. Reaching 20 µSv/h from 1 GBq at a metre takes 0.216 mm of lead. The tenth-value layer runs 5.0 times the half-value layer, not the 3.32 a single energy would give.

Half-life, specific activity and dose rate

Half-life15.84 minutes (950.4 s)
Decay modeisomeric transition
Specific activity2.41e+18 Bq/g (6.52e+7 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.0339 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.0339 mGy/h
Dose rate, 1 Ci at 1 m1.25 mGy/h
Kerma-weighted mean photon energy150.2 keV

10 lines above the cutoff, and what each contributes

2 further lines below the 20 keV cutoff, the highest at 16.27 keV and 58.0% emission probability in all, are excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
171.594828.73
146.7836.4818.02
184.952415.76
57.5346.888311.89
318.406.728.36
56.2826.895136.92
66.0719.700174.95
65.3115.511953.89
66.984.188231.06
356.470.2880.41

0.297 mm of lead halves this spectrum

Solved numerically across all 10 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead0.2971.474.95
tungsten0.2271.104.84
iron2.9715.35.15
copper2.3012.45.38
concrete18.265.93.62
water43.81493.42
aluminum15.858.33.70

A single energy would give 3.32. What a spread of energies does instead.

Activity over the first hours

Ten half-lives is 2.64 hours, so the activity moves measurably while a count is running: every figure has to carry the time it was referred to. The mean life 1/λ is 22.9 minutes.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity52.6 minutes
Time to fall to 1 %1.75 hours
Time to fall to 0.1 %2.63 hours

Limits of these dose rates

Gamma and decay calculators for Ta-182m2

Other Tantalum nuclides: Ta-182, Ta-182m1

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.