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Ba-133m shielding — lead half-value layer and dose rate

Barium-133m

Ba-133m · Barium, Z = 56, A = 133 · isomeric state m

Barium-133m (Ba-133m) carries 2.24e+16 Bq/g, or 6.06e+5 Ci/g: a gigabecquerel is 44.6 ng, no weighable quantity at all. It decays by isomeric transition with a half-life of 38.93 hours, which leaves 5.02% of today's activity after a week and 1.3e-15% after three months.

At 0.0178 mGy·m²/(GBq·h) the air kerma rate constant is 4.3× less than Cs-137 and 17× less than Co-60, placing it 58 of 96 photon emitters in this dataset. 1 GBq at 1 m reads 0.0178 mGy/h, and 1 Ci at the same distance 0.658 mGy/h.

11 lines clear the 20 keV cutoff, but 4 of them carry 90% of the dose rate. The leading one is 275.9 keV at 35.7% of the total — its emission probability is 17.7%, which is lower than the 28.8% of the 32.2 keV line it outranks.

Shielding barely arises: 0.0547 mm of lead halves the air kerma rate and 2.31 mm takes it to a tenth, thicknesses a source capsule is likely to exceed on its own. Steel does the halving in 0.301 mm. At 1 GBq and a metre it is already under 20 µSv/h with nothing in the way. The tenth-value layer runs 42.3 times the half-value layer, not the 3.32 a single energy would give.

Half-life, specific activity and dose rate

Half-life38.93 hours (1.401e+5 s)
Decay modeisomeric transition
Specific activity2.24e+16 Bq/g (6.06e+5 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.0178 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.0178 mGy/h
Dose rate, 1 Ci at 1 m0.658 mGy/h
Kerma-weighted mean photon energy120.1 keV

11 lines above the cutoff, and what each contributes

2 further lines below the 20 keV cutoff, the highest at 12.33 keV and 18.0% emission probability in all, are excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
275.9317.735.65
32.1928.830.13
31.8215.616.68
36.8310.68.69
36.488.57.09
37.262.131.71
632.590.01030.05
30.970.003880.00
30.630.00210.00
35.410.001410.00
35.090.001130.00

0.0547 mm of lead halves this spectrum

Solved numerically across all 11 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead0.05472.3142.27
tungsten0.04291.7039.62
iron0.30113.946.17
copper0.20011.959.44
concrete6.6748.97.34
water28.61164.07
aluminum5.0943.88.62

A single energy would give 3.32. What a spread of energies does instead.

Activity over days and weeks

Ten half-lives is 16.2 days — a storage problem rather than a disposal one, with 1.6e-66% of today's activity still there after a year. The mean life 1/λ is 2.34 days.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity5.39 days
Time to fall to 1 %10.8 days
Time to fall to 0.1 %16.2 days

Limits of these dose rates

Gamma and decay calculators for Ba-133m

Other Barium nuclides: Ba-133, Ba-137m

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.