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Ba-137m shielding — lead half-value layer and dose rate

Barium-137m

Ba-137m · Barium, Z = 56, A = 137 · isomeric state m

Barium-137m (Ba-137m) carries 1.99e+19 Bq/g, or 5.38e+8 Ci/g: a gigabecquerel is 50.2 pg, no weighable quantity at all. It decays by isomeric transition with a half-life of 2.552 minutes, which leaves 1.4e-168% of today's activity after a day and 0% after a week.

1 GBq at 1 m reads 0.0815 mGy/h, and 1 Ci at the same distance 3.02 mGy/h, from an air kerma rate constant of 0.0815 mGy·m²/(GBq·h) — 1.1× Cs-137 and 3.8× less than Co-60, and 26 of 96 among the photon emitters carried here.

6 lines clear the 20 keV cutoff, but one of them carries 90% of the dose rate. The leading one is 661.7 keV at 98.1% of the total — its emission probability is 89.9%, which is also the highest.

This is a shield that has to be designed: 5.34 mm of lead for a factor of two and 18.1 mm for a factor of ten, or 11.7 mm of steel to halve it, at which point the mass of the shield is part of the problem. Reaching 20 µSv/h from 1 GBq at a metre takes 11.0 mm of lead.

Half-life, specific activity and dose rate

Half-life2.552 minutes (153.1 s)
Decay modeisomeric transition
Specific activity1.99e+19 Bq/g (5.38e+8 Ci/g)
Air kerma rate constant Γ (δ = 20 keV)0.0815 mGy·m²/(GBq·h)
Dose rate, 1 GBq at 1 m0.0815 mGy/h
Dose rate, 1 Ci at 1 m3.02 mGy/h
Kerma-weighted mean photon energy649.8 keV

662 keV carries 98% of the dose rate

1 further line below the 20 keV cutoff, the highest at 4.97 keV and 0.966% emission probability in all, is excluded here and from Γ. Why the two columns rank differently.

Energy (keV)Emission probability (%)Share of dose rate (%)
661.6689.998.11
32.193.871140.88
31.822.101250.49
36.831.425610.26
36.481.138670.21
37.260.286940.05

5.34 mm of lead halves this spectrum

Solved numerically across all 6 lines, narrow beam. Why not one representative energy.

MaterialHVL (mm)TVL (mm)TVL / HVL
lead5.3418.13.39
tungsten3.5412.03.39
iron11.739.53.39
copper10.435.13.39
concrete37.21263.39
water79.02663.37
aluminum33.51133.39

A single energy would give 3.32. What a spread of energies does instead.

Activity over the first hours

Ten half-lives is 25.5 minutes, so the activity moves measurably while a count is running: every figure has to carry the time it was referred to. The mean life 1/λ is 3.68 minutes.

ElapsedFraction remaining
1 half-life50.0 %
2 half-lives25.0 %
5 half-lives3.13 %
10 half-lives0.0977 %
Time to fall to 10 % of today's activity8.48 minutes
Time to fall to 1 %17.0 minutes
Time to fall to 0.1 %25.4 minutes

Limits of these dose rates

Gamma and decay calculators for Ba-137m

Other Barium nuclides: Ba-133, Ba-133m

Computed from the IAEA Nuclear Data Section — Livechart API (ENSDF) and the NIST X-Ray Mass Attenuation Coefficients. Derivations and citations.